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Piezoelectric materials are widely used as electromechanical couples for a variety of sensors and actuators in nanoscale electronic devices. The majority of piezoelectric devices display lateral patterning of counter electrodes beside active materials such as two-dimensional transition metal dichalcogenides (2D TMDs). As a result, their piezoelectric output response is strongly dependent on the lattice orientation of the 2D TMD crystal structure, limiting their piezoelectric properties. To overcome this issue, we fabricated a vertical sandwich design of a piezoelectric sensor with a conformal contact to enhance the overall piezoelectric performance. In addition, we enhanced the piezoelectric properties of 2D WS 2 by carrying out a unique solvent-vapor annealing process to produce a sulfur-deficient WS 2 (1-x) structure that yielded a 3-fold higher piezoelectric response voltage (96.74 mV) than did pristine WS 2 to a 3 …